Document Type

Article

Publication Date

7-14-2023

Journal / Book Title

ACS Applied Polymer Materials

Abstract

Silk, a popular biomaterial, is used as a greener alternative of toxic reducing agent in biocompatible graphene synthesis. However, silk often forms gel uncontrollably due to its heavy-chain molecular weight and faces significant challenges in the reduction, stabilization, and dispersion process of graphene. In this contribution, we report a rapid chemical synthesis approach for a low-molecular-weight silk-inspired polymer via ring-opening and microwave-assisted Diels-Alder-aided step-growth polymerizations. This synthetic polymer with periodic sequences of hydrophilic and hydrophobic moieties not only reduces graphene oxide efficiently but also enhances the dispersibility of hydrophobic reduced graphene oxide in aqueous media.

DOI

10.1021/acsapm.3c00353

Rights

This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/).

Published Citation

Valmonte, Z., Baker, Z., Loor, J., & Sarkar, A. (2023). Concurrent Reduction and Stabilization of Graphene Oxide Dispersion by Silk-Inspired Polymer. ACS applied polymer materials, 5(7), 4621–4627. https://doi.org/10.1021/acsapm.3c00353

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Chemistry Commons

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